Faculty Bibliography

The validation of human biological models for inhaled radionuclides is nearly impossible. Requirements for validation are: (1) the measurement of the relevant human tissue data and (2) valid exposure measurements over the interval known to apply to tissue uptake. Two lung models, ICRP 30(( 1)) and ICRP 66(( 2)), are widely used to estimate lung doses following acute occupational or environmental exposure. Both ICRP 30 and 66 lung models are structured to estimate acute rather than chronic exposure. Two sets of human tissue measurements are available: (210)Po accumulated in tissue from inhaled cigarettes and ingested in diet and airborne global fallout (239,240)Pu accumulated in the lungs from inhalation. The human tissue measurements include pulmonary and bronchial tissue in smokers, ex-smokers and non-smokers analysed radiochemically for (210)Po, and pulmonary, bronchial and lymph nodes analysed for (239,240)Pu in lung tissue collected by the New York City Medical Examiner from 1972 to 1974. Both ICRP 30 and 66 models were included in a programme to accommodate chronic uptake. Neither lung model accurately described the estimated tissue concentrations but was within a factor of 2 from measurements. ICRP 66 was the exception and consistently overestimated the bronchial concentrations probably because of its assumption of an overly long 23-d clearance half-time in the bronchi and bronchioles.

ABSTRACT: To provide detailed information for bronchial dose estimates, aerosol particle size distributions, and radon gas concentration, measurements were made in six residential homes and three laboratory rooms in different office buildings in the city of Ottawa. In the literature, most particle size distribution measurements are taken with samplers operating for a few days at most. In this study, the particle size samplers collected the samples from 77 to 162 d. The equilibrium factor determined from the long-term measurements ranged from 0.6 to almost 1 with an average of 0.75. Even though radon concentrations were quite different between residential setting and office buildings, the average equilibrium factor was similar in the two different indoor environments. The results suggest that at least in some basements, if they were occupied, the radon dose would be about twice as high as normally estimated from the conventional Feq value of 0.4.

ABSTRACT: An intercomparison on thoron (Rn) measurement was carried out between National Institute of Radiological Sciences, Japan (NIRS), and New York University School of Medicine, USA (NYU). The measurements of Rn concentration at NIRS and NYU were performed by using the scintillation cell method and the two-filter method, respectively, as the standard measurement method. Three types of alpha track detectors based on passive radon (Rn)-Rn discriminative measurement technique were used: Raduet and Radopot detectors were used at NIRS, and four-leaf detectors were used at NYU. In this study, the authors evaluated Rn concentration variation in terms of run for exposure, measurement method, and exposure chamber. The detectors were exposed to Rn gas with approximately 15 kBq m during the period from 0.75 to 3 d. As a result, the variation of each measurement method among these exposure runs was comparable to or less than that for the two-filter method. Agreement between the standard measurement methods of NIRS and NYU was observed to be about 10%, as is the case with the passive detectors. The Raduet detector showed a large variation in the detection response between the NIRS and NYU chambers, which could be related to different traceability.

An exploratory radon measurement in 1990 identified 190 Bq m(-3) in the basement of a newly built home in Central New Jersey. Subsequently, the owner had a sub-slab remediation system installed in the basement, i.e. PVC duct through the basement floor connecting to an exhaust fan venting to the house roof. Sequential radon measurements began in 1992 using the NYU alpha-track detector. The homeowner wanted to insure the long-term durability of this remedial system. Seventeen years of measurements show the system functioned properly and reduced an established baseline concentration of 370+/-8, 56+/-1 and 67+/-1 Bq m(-3) for the basement, first and second floors, respectively, to an average of 19+/-4, 13+/-3 and 10+/-0.1 Bq m(-3). The last measurement, 2007-2008, with a newer NYU detector measured both (222)Rn (radon) and (220)Rn (thoron). The basement thoron concentration was 1.5+/-0.9 Bq m(-3) or about 8 % of the (222)Rn value

A miniature four-chamber alpha track detector was developed that measures both (222)Rn (radon) and (220)Rn (thoron), in duplicate. Using this detector and the previous long-term measurements of the (220)Rn decay products (212)Pb, and (212)Bi, an equilibrium factor, F(eq), is derived for both outdoor and indoor (220)Rn environments (0.004+/-0.001 outdoors and 0.04+/-0.01 indoors). The lung airway dose can then be calculated from a dose factor from UNSCEAR that requires the equilibrium equivalent thoron concentration (EEC), i.e. the product of F(eq) and the (220)Rn gas concentration. The lung dose from thoron in domestic or occupational surveys is often overlooked. The values of F(eq) for thoron in several published studies are in general agreement with the values reported here. Thus, a long-term alpha track measurement of thoron multiplied by an appropriate indoor or outdoor equilibrium factor yields the EEC, which can be used to assess bronchial lung dose

A roundtable discussion was made at the end of the workshop. All the presentations were summarised in this discussion. It involved measurement techniques, quality assurance and dose assessment and health effects of thoron and its progeny. In particular, major epidemiological studies may be affected by thoron interference in radon measurements. Since their data are not sufficient when compared with that of radon, further efforts in thoron studies will be needed.